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Angewandte Chemie International Edition
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Dearomative [3,3]‐Claisen Rearrangement of 2‐Indolyl Alcohols: An Efficient and General Protocol for Synthesizing 3,3‐Disubstituted Indolines and Related Indole Alkaloids
2 days ago
This work presents a practical dearomative [3,3]-Claisen rearrangement of 2-indolyl alcohols, enabling...
Interfacial Electronic Modulation Redirects Anodic Radical Chemistry for Selective C─C Bond Cleavage in Electro‐Oxidative Lignin Depolymerization
2 days ago
We propose a CuO/Cu0.92Co2.08O4 heterocatalyst that achieves 88% conversion of 2-phenoxy-1-phenylethanol to...
Single‐Molecule Additive Integrating Na‐Ion Reservoir, Cosolvent, and Diluent Functions for Low‐Temperature Na‐Ion Batteries
2 days ago
NaB(C2H5)4 was dissolved in the electrolyte and underwent complete decomposition below 4.0...
CO2‐Derived Degradable Polythioester Adhesives From Proton‐Trap‐Assisted S/O Isomerization‐Driven Cationic Ring‐Opening Polymerization
2 days ago
This work presents a proton-trap-assisted S/O isomerization-driven cationic ring-opening polymerization of the...
Substrate‐Controlled Dearomative Cycloadditions of Perfluoronaphthalenes via Visible‐Light Energy Transfer Catalysis: Switchable Access to [2+2], [4+2], and Diastereoconvergent Cycloadducts
2 days ago
Visible-light energy-transfer catalysis enables olefin-controlled intermolecular dearomative cycloaddition of polyfluoronaphthalenes, switching between...
Reactivity of a d2 Mo(IV) Alkylidyne Fragment Bearing a PNCNP Pincer Ligand Toward Alkynes: Coordination and Catalytic Alkyne Metathesis
2 days ago
Novel Mo carbyne-alkyne complexes were synthesized and fully characterized. Incorporation of N-Me...
Extended Endocyclic Conjugation and N,N‐Bidentate Chelation Alleviate the Capacity–Stability Trade‐Off in Organic Magnesium Battery Cathodes
2 days ago
A rational molecular design is established by combining extended endocyclic π-conjugation and...
Beyond Fluorination: A Golden Criterion Guided by Chemical Coordination‐Informed Machine Learning for High‐Voltage Electrolyte Design
2 days ago
By using Chemical Coordination‑Informed feature parsing that quantifies atomic molarities in specific...
Interfacial Proton Ordering Near the Electrode Surface Directs Carbonyl Electroreduction to Methylene
2 days ago
Interfacial proton ordering near the electrode interface transforms alcohol intermediates from dead-end...
Protonation‐Triggered Unlocking of Interlayer Carbon Nitride for Rapid Nanosheet Preparation
2 days ago
Triflic-acid-mediated protonation unlocks interlayer interactions in bulk g-C3N4, enabling mild, rapid exfoliation...
Precise Regulation of Intrachannel Negative Charge Density in Metal‐Organic Frameworks for Efficient Alkali‐Ion Transport
2 days ago
In this study, MOFs with tunable channel charge densities were engineered to...
Spatial Evolution of Coke in ZSM‐5 Catalysts During Methanol‐to‐Hydrocarbons Conversion Revealed by In Situ X‐Ray Photoelectron Spectroscopy
2 days ago
Coking is the central source of deactivation of zeolite catalysts. Using in...